TY - JOUR
T1 - Giant magnetoresistance, Fermi-surface topology, Shoenberg effect, and vanishing quantum oscillations in the type-II Dirac semimetal candidates MoSi2 and WSi2
AU - Pavlosiuk, Orest
AU - Swatek, Przemysław Wojciech
AU - Wang, Jian Ping
AU - Wiśniewski, Piotr
AU - Kaczorowski, Dariusz
N1 - Publisher Copyright:
© 2022 American Physical Society.
PY - 2022/2/15
Y1 - 2022/2/15
N2 - We performed comprehensive theoretical and experimental studies of the electronic structure and the Fermi surface topology of two novel quantum materials, MoSi2 and WSi2. The theoretical predictions of the electronic structure in the vicinity of the Fermi level was verified experimentally by thorough analysis of the observed quantum oscillations in both electrical resistivity and magnetostriction. We established that the Fermi surface sheets in MoSi2 and WSi2 consist of 3D dumbbell-shaped holelike pockets and rosette-shaped electronlike pockets, with nearly equal volumes. Based on this finding, both materials were characterized as almost perfectly compensated semimetals. In conjunction, the magnetoresistance attains giant values of 104 and 105% for WSi2 and MoSi2, respectively. In turn, the anisotropic magnetoresistance achieves -95% and -98% at T=2 K and in B=14 T for WSi2 and MoSi2, respectively. Furthermore, for both compounds we observed the Shoenberg effect in their Shubnikov-de Haas oscillations that persisted at as high temperature as T=25 K in MoSi2 and T=12 K in WSi2. In addition, we found for MoSi2 a rarely observed spin-zero phenomenon. Remarkably, the electronic structure calculations revealed type-II Dirac cones located near 480 and 710 meV above the Fermi level in MoSi2 and WSi2, respectively.
AB - We performed comprehensive theoretical and experimental studies of the electronic structure and the Fermi surface topology of two novel quantum materials, MoSi2 and WSi2. The theoretical predictions of the electronic structure in the vicinity of the Fermi level was verified experimentally by thorough analysis of the observed quantum oscillations in both electrical resistivity and magnetostriction. We established that the Fermi surface sheets in MoSi2 and WSi2 consist of 3D dumbbell-shaped holelike pockets and rosette-shaped electronlike pockets, with nearly equal volumes. Based on this finding, both materials were characterized as almost perfectly compensated semimetals. In conjunction, the magnetoresistance attains giant values of 104 and 105% for WSi2 and MoSi2, respectively. In turn, the anisotropic magnetoresistance achieves -95% and -98% at T=2 K and in B=14 T for WSi2 and MoSi2, respectively. Furthermore, for both compounds we observed the Shoenberg effect in their Shubnikov-de Haas oscillations that persisted at as high temperature as T=25 K in MoSi2 and T=12 K in WSi2. In addition, we found for MoSi2 a rarely observed spin-zero phenomenon. Remarkably, the electronic structure calculations revealed type-II Dirac cones located near 480 and 710 meV above the Fermi level in MoSi2 and WSi2, respectively.
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U2 - 10.1103/PhysRevB.105.075141
DO - 10.1103/PhysRevB.105.075141
M3 - Article
AN - SCOPUS:85126070991
SN - 2469-9950
VL - 105
JO - Physical Review B
JF - Physical Review B
IS - 7
M1 - 075141
ER -