Impacts of catalyst coating on the filtration performance of catalyzed wall-flow filters: From the viewpoint of microstructure

Qiang Lyu; Qisheng Ou; Weiqi Chen; Yujun Wang; Cheng Chang; Yuejin Li; Defu Che; David Y.H. Pui

doi:10.1016/j.seppur.2021.120417

Impacts of catalyst coating on the filtration performance of catalyzed wall-flow filters: From the viewpoint of microstructure

Qiang Lyu, Qisheng Ou, Weiqi Chen, Yujun Wang, Cheng Chang, Yuejin Li, Defu Che, David Y.H. Pui

Research output: Contribution to journal › Article › peer-review

7 Scopus citations

Abstract

Initial filtration efficiency and soot loading characteristics are important performance criteria for catalyzed wall-flow filters. In this context, the influence of catalyst coating on filtration performance was investigated over a set of bare and coated silicon carbide (SiC) filter cores. Catalyst coating demonstrates a significant decrease effect on the initial filtration efficiency. Both filtration efficiency and pressure drop increase faster with time on coated filters in the deep-bed filtration regime. The scanning electron microscopy (SEM) results reveal that catalyst is preferentially deposited in the smaller pores. The mercury intrusion porosimetry (MIP) data show that catalyst coating reduces the pore volume for the pores relevant to filtration. The capillary flow porometry (CFP) results confirm that the coated catalyst wipes out a group of smaller pores. Accordingly, for the first time, we provide a working mechanism to explain the decreased filtration efficiency on catalyzed filters based on the experimental results and characterization data.

Original language	English (US)
Article number	120417
Journal	Separation and Purification Technology
Volume	285
DOIs	https://doi.org/10.1016/j.seppur.2021.120417
State	Published - Mar 15 2022
Externally published	Yes

Bibliographical note

Funding Information:
The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc. BASF Corporation, Boeing Company, Corning Co. China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc. Donaldson Company, Inc. Entegris, Inc. Ford Motor Company, Guangxi WatYuan Filtration System Co. Ltd, LG Electronics Inc. Parker Hannifin, Samsung Electronics Co. Ltd. Xinxiang Shengda Filtration Technology Co. Ltd. TSI Inc. W. L. Gore & Associates, Inc. Shigematsu Works Co. Ltd. and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073).

Funding Information:
The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc., BASF Corporation, Boeing Company, Corning Co., China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc., Donaldson Company, Inc., Entegris, Inc., Ford Motor Company, Guangxi WatYuan Filtration System Co., Ltd, LG Electronics Inc., Parker Hannifin, Samsung Electronics Co., Ltd., Xinxiang Shengda Filtration Technology Co., Ltd., TSI Inc., W. L. Gore & Associates, Inc., Shigematsu Works Co., Ltd., and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073).

Publisher Copyright:
© 2022 Elsevier B.V.

Keywords

Catalyst coating
Catalyzed soot filter
Engine exhaust
Filtration performance
Pore size distribution

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title = "Impacts of catalyst coating on the filtration performance of catalyzed wall-flow filters: From the viewpoint of microstructure",

abstract = "Initial filtration efficiency and soot loading characteristics are important performance criteria for catalyzed wall-flow filters. In this context, the influence of catalyst coating on filtration performance was investigated over a set of bare and coated silicon carbide (SiC) filter cores. Catalyst coating demonstrates a significant decrease effect on the initial filtration efficiency. Both filtration efficiency and pressure drop increase faster with time on coated filters in the deep-bed filtration regime. The scanning electron microscopy (SEM) results reveal that catalyst is preferentially deposited in the smaller pores. The mercury intrusion porosimetry (MIP) data show that catalyst coating reduces the pore volume for the pores relevant to filtration. The capillary flow porometry (CFP) results confirm that the coated catalyst wipes out a group of smaller pores. Accordingly, for the first time, we provide a working mechanism to explain the decreased filtration efficiency on catalyzed filters based on the experimental results and characterization data.",

keywords = "Catalyst coating, Catalyzed soot filter, Engine exhaust, Filtration performance, Pore size distribution",

author = "Qiang Lyu and Qisheng Ou and Weiqi Chen and Yujun Wang and Cheng Chang and Yuejin Li and Defu Che and Pui, {David Y.H.}",

note = "Funding Information: The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc. BASF Corporation, Boeing Company, Corning Co. China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc. Donaldson Company, Inc. Entegris, Inc. Ford Motor Company, Guangxi WatYuan Filtration System Co. Ltd, LG Electronics Inc. Parker Hannifin, Samsung Electronics Co. Ltd. Xinxiang Shengda Filtration Technology Co. Ltd. TSI Inc. W. L. Gore & Associates, Inc. Shigematsu Works Co. Ltd. and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073). Funding Information: The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc., BASF Corporation, Boeing Company, Corning Co., China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc., Donaldson Company, Inc., Entegris, Inc., Ford Motor Company, Guangxi WatYuan Filtration System Co., Ltd, LG Electronics Inc., Parker Hannifin, Samsung Electronics Co., Ltd., Xinxiang Shengda Filtration Technology Co., Ltd., TSI Inc., W. L. Gore & Associates, Inc., Shigematsu Works Co., Ltd., and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073). Publisher Copyright: {\textcopyright} 2022 Elsevier B.V.",

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AU - Ou, Qisheng

AU - Chen, Weiqi

AU - Wang, Yujun

AU - Chang, Cheng

AU - Li, Yuejin

AU - Che, Defu

AU - Pui, David Y.H.

N1 - Funding Information: The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc. BASF Corporation, Boeing Company, Corning Co. China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc. Donaldson Company, Inc. Entegris, Inc. Ford Motor Company, Guangxi WatYuan Filtration System Co. Ltd, LG Electronics Inc. Parker Hannifin, Samsung Electronics Co. Ltd. Xinxiang Shengda Filtration Technology Co. Ltd. TSI Inc. W. L. Gore & Associates, Inc. Shigematsu Works Co. Ltd. and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073). Funding Information: The authors thank the support of members of the Center for Filtration Research: 3 M Corporation, Applied Materials, Inc., BASF Corporation, Boeing Company, Corning Co., China Yancheng Environmental Protection Science and Technology City, Cummins Filtration Inc., Donaldson Company, Inc., Entegris, Inc., Ford Motor Company, Guangxi WatYuan Filtration System Co., Ltd, LG Electronics Inc., Parker Hannifin, Samsung Electronics Co., Ltd., Xinxiang Shengda Filtration Technology Co., Ltd., TSI Inc., W. L. Gore & Associates, Inc., Shigematsu Works Co., Ltd., and the affiliate member National Institute for Occupational Safety and Health (NIOSH). The authors also acknowledge the support from the program of China Scholarship Council (CSC201806280073). Publisher Copyright: © 2022 Elsevier B.V.

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Y1 - 2022/3/15

N2 - Initial filtration efficiency and soot loading characteristics are important performance criteria for catalyzed wall-flow filters. In this context, the influence of catalyst coating on filtration performance was investigated over a set of bare and coated silicon carbide (SiC) filter cores. Catalyst coating demonstrates a significant decrease effect on the initial filtration efficiency. Both filtration efficiency and pressure drop increase faster with time on coated filters in the deep-bed filtration regime. The scanning electron microscopy (SEM) results reveal that catalyst is preferentially deposited in the smaller pores. The mercury intrusion porosimetry (MIP) data show that catalyst coating reduces the pore volume for the pores relevant to filtration. The capillary flow porometry (CFP) results confirm that the coated catalyst wipes out a group of smaller pores. Accordingly, for the first time, we provide a working mechanism to explain the decreased filtration efficiency on catalyzed filters based on the experimental results and characterization data.

AB - Initial filtration efficiency and soot loading characteristics are important performance criteria for catalyzed wall-flow filters. In this context, the influence of catalyst coating on filtration performance was investigated over a set of bare and coated silicon carbide (SiC) filter cores. Catalyst coating demonstrates a significant decrease effect on the initial filtration efficiency. Both filtration efficiency and pressure drop increase faster with time on coated filters in the deep-bed filtration regime. The scanning electron microscopy (SEM) results reveal that catalyst is preferentially deposited in the smaller pores. The mercury intrusion porosimetry (MIP) data show that catalyst coating reduces the pore volume for the pores relevant to filtration. The capillary flow porometry (CFP) results confirm that the coated catalyst wipes out a group of smaller pores. Accordingly, for the first time, we provide a working mechanism to explain the decreased filtration efficiency on catalyzed filters based on the experimental results and characterization data.

KW - Catalyst coating

KW - Catalyzed soot filter

KW - Engine exhaust

KW - Filtration performance

KW - Pore size distribution

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DO - 10.1016/j.seppur.2021.120417

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SN - 1383-5866

VL - 285

JO - Separation and Purification Technology

JF - Separation and Purification Technology

M1 - 120417

ER -

Impacts of catalyst coating on the filtration performance of catalyzed wall-flow filters: From the viewpoint of microstructure

Abstract

Bibliographical note

Keywords

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